Unveiling charge dynamics on the generation of high extinction wide pulse generation on thin-film lithium tantalate

Abstract

We experimentally demonstrate high-extinction optical pulse generation in thin-film lithium tantalate (TFLT), achieving a wide range of pulse widths with sharp rise and fall edges, without measurable distortion or long temporal tails. We further provide a direct one-to-one comparison with thin-film lithium niobate (TFLN) modulators under identical measurement conditions. Our results reveal that the distorted pulse response observed in TFLN originates from charge activation and transport, whereas the distortion-free response in TFLT is enabled by the substantially larger activation energy of defect-related charge carriers. This larger activation barrier suppresses leakage-current-induced charging dynamics, thereby enabling stable and distortion-free pulse generation. The successful generation of high-extinction, distortion-free optical pulses in TFLT can play a significant role in integrated quantum photonic technologies, particularly for qubit preparation, measurement, and fast feedback circuits.